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Three-dimension (3D) graphene made by CVD has recently raised increasing attentions due to its unique 3D porous structure, excellent physical properties and potential applications. Most of the recent works focus on Ni foam-based 3D graphene and their composites. However, it is limited in the yield and the mechanical strength required in some realistic applications. Therefore, it is significant to exploit a technique to obtain rapidly high-density three-dimension graphene macroscopic objects (3D-GMOs) for the promising applications.